Quantum coherence controls the charge separation in a prototypical artificial light harvesting system
- Falke S. M.
- Rozzi C. A.
- Spallanzani N.
- Rubio A.
- Molinari E.
- Brida D.
- Maiuri M.
- Cerullo G.
- Schramm H.
- Christoffers J.
- Lienau C.
DOIAbstract
Ultrafast spectroscopy and quantum-dynamics simulations of an artificial supramolecular light-harvesting system - a supramolecular triad - provide strong evidence that the quantum-correlated wavelike motion of electrons and nuclei on a timescale of few tens of femtoseconds governs the ultrafast electronic charge transfer. © Owned by the authors, published by EDP Sciences, 2013
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