The international Phébus FP programme was initiated in 1988 by the French "Institut de Radioprotection et de Sûreté Nucléaire" (IRSN2), in cooperation with the European Commission (EC), to investigate key phenomena involved in light water reactor (LWR) severe accidents. In addition to IRSN and EC, other partner countries contributed to this programme. The Phébus facility was operated by the French "Commissariat à l'Energie Atomique" (CEA) at Cadarache, providing prototypic reactor conditions which allowed to study fuel degradation, the release of fission products (FPs) and their transport and behaviour through the reactor coolant system (RCS) and in the containment building. A specific attention was paid to iodine radiochemistry due to its ...