The international Phébus FP (fission product) programme investigated core degradation and radioactive product release originating from a core melt-down accident in Light Water Reactors. Five integral in-pile tests were performed at Cadarache. During these tests, the main processes which affect the severe degradation of fuel and control rods, the release of fission products and control materials, their transport through the reactor coolant circuit as well as their deposition as aerosols in the containment vessel were assessed. Various physico-chemical processes such as aerosol agglomeration and various deposition modes, such as gravitational settling, diffusiophoresis and deposition on the stainless steel walls were analysed during each test...