This thesis is a contribution to the field of algebraic cryptanalysis. Specifically the following topics have been studied: We construct and analyze Feistel and SLN ciphers that have a sound design strategy against linear and differential cryptanalysis. The encryption process for these cipher can be described by very simple polynomial equations. For a block and key size of 128 bits, we present ciphers for which practical Gröbner Basis Attacks can recover the full cipher key for up to 12 rounds requiring only a minimal number of plaintext/ciphertext pairs. We show how Gröbner bases for a subset of these ciphers can be constructed with negligible computational effort. This reduces the key-recovery problem to a Gröbner basis conversion problem...