The need for computing functions of large, sparse matrices arises in Bayesian spatial models where the computations using Gaussian Markov random fields require the evaluation of G -1 and G -1/2 for the precision matrix G and in the geostatistical approach where approximations of R -1 and R 1/2 are needed for the covariance matrix R . In both cases, good approximations to the desired matrix functions are required over a range of probable values of a vector v drawn randomly from a given population, as occurs in simulation techniques for finding posterior distributions such as Markov chain Monte Carlo. Consequently, it is preferable that the complete matrix function approximation be determined rather than for its action on a ...