This thesis is an argument for the view that there are problems for Modal Reductionism, the thesis that modality can satisfactorily be defined in non-modal terms. I proceed via a case study of David Lewis’s theory of concrete possible worlds. This theory is commonly regarded as the best and most influential candidate reductive theory of modality. Based on a detailed examination of its ontology, analysis and justification, I conclude that it does badly with respect to the following four minimal conditions on a satisfactory reductive theory of modality: that it be (a) genuinely reductive, (b) materially adequate, (c) conceptually adequate and (d) that i...