Highly customisable implants with lattice structures can be achieved using selective laser melting (SLM) paving the way for tailored biodegradable Fe-based implants. For the first time, a systematic analysis is presented in terms of laser processing conditions required for scaffolds of pure Fe and a binary Fe-35 Mn alloy. The processability of the two materials were compared in terms of densification behaviour, surface roughness and geometrical error. Both materials were successfully processed into high quality scaffolds with excellent strut morphology and low processing porosity. The differences in the laser processing conditions between the pure metal and the binary alloy were discussed. The lower melting temperature of the Fe-35 Mn alloy...