AbstractLet A be a commutative ring with identity. Loday [14] and others have described the multiplicative structure (both graded and ungraded) on the higher algebraic K-theory of A. In [19] and [24], Quillen has indicated the existence of a λ-ring structure on the “K-cohomology” groups K(X, A)=[X, K0(A)×BGL(A)+].The purpose of this paper is to develop some of this structure and show how it can be useful in obtaining information about the K-groups themselves. In particular, standard techniques will then allow one to construct Adams operationsψk in algebraic K-theory. These operations enjoy some of the attractive properties of their counterparts in the K-theory of complex vector bundles over a finite complex. Indeed, with this machinery and ...