This thesis addresses four fundamental, yet unresolved, issues in brittle fracture mechanics: (a) the validity of linear elasticity in the crack-tip region, (b) crack growth direction under mixed-mode loading, (c) the nature and impact of cohesive stresses, (d) the effect of crack-face friction on the crack growth criterion in Griffith’s model for compressive failure. It is a well known fact that, according to classical elasticity, the stress in the near-tip region of the crack is singular, which has led to a debate over the validity of linear elasticity in this region. The strain, stress and elastic strain energy of a cracked silicon crystal in the crack-tip region is calculated, according to atomistic simulations, and compared to the c...