Aerosol optical properties from columnar data during the second Aerosol Characterization Experiment on the south coast of Portugal

Measurements of aerosol optical properties over the atmospheric column (aerosol optical thickness, spectral angular sky radiance (sky brightness), and downwelling hemispheric flux) have been used to derive climate-relevant aerosol parameters such as the phase function, the broadband single-scattering albedo, and the refractive index. These parameters are needed to estimate the direct short-wave radiative forcing by aerosols and to validate aerosol models in the satellite retrieval algorithms. Values of the broadband single-scattering albedo obtained in this study range between w0 = 0.98 (marine aerosols) and 0.90 (continental pollution aerosols). The columnar ambient broadband refractive index is found to be m = 1.39 ± 0.044 i (