International audienceSpectral photon-counting CT offers novel potentialities to achieve quantitative decomposition of material components, in comparison with traditional energy-integrating CT or dual-energy CT. Nonetheless, achieving accurate material decomposition, especially for low-concentration materials, is still extremely challenging for current sCT, due to restricted energy resolution stemming from the trade-off between the number of energy bins and undesired factors such as quantum noise. We propose to improve material decomposition by introducing the notion of super-energy-resolution in sCT. The super-energyresolution material decomposition consists in learning the relationship between simulation and physical phantoms in image dom...