Impacts of Household Characteristics, Activities and Building Characteristics on Indoor Concentrations of Semi-volatile Organic Compounds

When compared to outdoors, the indoor environment often has higher concentrations of some SVOCs, such as brominated flame retardants (BFRs), organophosphate esters (OPEs) and phthalates that are used as additive flame retardants and plasticizers from consumer products and building materials. Some outdoor SVOCs, such as polycyclic aromatic hydrocarbons (PAHs), can be transported into indoor environments, increasing indoor exposures to these compounds. With the increasing concerns about the implications of exposure for human health, attention has turned towards concentrations of SVOCs in indoor environments, particularly in residential dwellings where North Americans spend more than 60% of their time. This thesis documented concentrations of these SVOCs in residential buildings, focussed on the exposure disparities in SVOCs according to socio-economic status (SES), and developed SVOC sampling methods in low-SES homes. Quantitative filter forensics (QFF) was extended to portable air cleaners with portable filters to quantitatively estimate indoor particle-bound SVOCs, overcoming the limitations of traditional QFF requiring forced-air heating, ventilation and air conditioning (HVAC) systems, while also improving indoor air quality by removing particular matter (PM). This thesis also advanced knowledge on the impacts of household characteristics, activities and building characteristics on indoor SVOC concentrations. The research found SVOC exposure disparities according to SES in Canada, reinforcing the importance of better understanding of the intersection between contaminant exposure, housing quality, household characteristics, and activities that can elevate SVOC levels, and SES, with the aim of reducing exposures from residences in an equitable manner.Ph.D