In this thesis we apply coalgebraic modelling to gain new insights into automata theory and modal logic. Briefly summarised, the main contributions consist of (i) a coalgebraic technique for synthesising Mealy machines from arithmetic bitstream specifications, and results that relate Mealy machines to rational specifications in terms of expressivity and complexity; (ii) a coalgebraic perspective on subsequential transducers, and a systematic classification of reflective subcategories of subsequential structures; (iii) bisimulation notions for neighbourhood structures and model theoretic results for classical modal logic, including interpolation and a characterisation of classical modal logic as the bisimulation invariant fragment of first o...