This paper presents an experimental study of the structural dynamics and the wake vortex modes of a lightly damped, elastically mounted cylinder undergoing vortex-induced vibration (VIV) in the transverse direction. The cylinder is neutrally buoyant with the mass ratio m* = 1.0, and has a low damping coefficient ζ = 0.0173. The influence of variation in the free-stream velocity (corresponding to the reduced velocity range 1.53 ≤ U* ≤ 6.62, or the Reynolds number range 3000 ≤ Re ≤ 13,000) on the structural dynamics of the cylinder is examined, in conjunction with detailed flow measurements around the cylinder using digital Particle Image Velocimetry (PIV). The cylinder is stationary at U* ≤ 2.55, and begins to vibrate at U* ≥ 3.05 (or in syn...