The influence of the atmospheric radon background on the airborne gamma spectrum can seriously affect researchers’ judgement of ground radiation information. However, due to load and endurance, unmanned aerial vehicle (UAV)-borne gamma-ray spectrometry is difficulty installing upward-looking detectors to monitor atmospheric radon background. In this paper, an advanced spectral-ratio method was used to correct the atmospheric radon background for a UAV-borne gamma-ray spectrometry in Inner Mongolia, China. By correcting atmospheric radon background, the ratio of the average count rate of U window in the anomalous radon zone (S5) to that in other survey zone decreased from 1.91 to 1.03, and the average uranium content in S5 decreased from 4.6...