In this contribution we present a theoretical analysis in which the frequency- and time-domain formalism of ultrafast nonlinear spectroscopy is thoroughly reexamined. The complete expressions valid even for single-cycle-pulse applications are derived for the nonlinear signal in the frequency and time domains. We also assert that the influence of geometrical delay smearing does not introduce a significant distortion of the observed traces provided that the geometry is carefully optimized. The derived formalism is applied to photon-echo spectroscopy on the hydrated electron with 5-fs pulses
The problem of measuring broad-band femtosecond pulses by the technique of second-harmonic generatio...
Chemical reaction dynamics and chemical rate processes in the liquid phase are intimately connected ...
Richard T. White, Yabai He, Brian J. Orr, Mitsuhiko Kono, and K. G. H. Baldwinhttp://www.opticsinfob...
In this contribution we present a theoretical analysis in which the frequency- and time-domain forma...
A very high temporal resolution and a broad bandwidth are but two advantages provided by the use of ...
Ultrafast four-wave mixing experiments using chirped-pulse excitation of a dye molecule in solution ...
Third-order optical nonlinearities play a vital role for generation1,2 and characterization 3-5 of s...
In this contribution we show that enhanced mode suppression can be obtained by time-gating the stimu...
Since the birth of mode-locking the temporal duration of optical pulses has radically diminished. In...
This dissertation reports a series of experiments directed towards nonlinear material characterizati...
This work describes the use of a broadband spectral source for nonlinear spectroscopy to characteriz...
In linear optics, light fields do not mutually interact in a medium. However, they do mix when their...
The problem of measuring broad-band femtosecond pulses by the technique of second-harmonic generatio...
Chemical reaction dynamics and chemical rate processes in the liquid phase are intimately connected ...
Richard T. White, Yabai He, Brian J. Orr, Mitsuhiko Kono, and K. G. H. Baldwinhttp://www.opticsinfob...
In this contribution we present a theoretical analysis in which the frequency- and time-domain forma...
A very high temporal resolution and a broad bandwidth are but two advantages provided by the use of ...
Ultrafast four-wave mixing experiments using chirped-pulse excitation of a dye molecule in solution ...
Third-order optical nonlinearities play a vital role for generation1,2 and characterization 3-5 of s...
In this contribution we show that enhanced mode suppression can be obtained by time-gating the stimu...
Since the birth of mode-locking the temporal duration of optical pulses has radically diminished. In...
This dissertation reports a series of experiments directed towards nonlinear material characterizati...
This work describes the use of a broadband spectral source for nonlinear spectroscopy to characteriz...
In linear optics, light fields do not mutually interact in a medium. However, they do mix when their...
The problem of measuring broad-band femtosecond pulses by the technique of second-harmonic generatio...
Chemical reaction dynamics and chemical rate processes in the liquid phase are intimately connected ...
Richard T. White, Yabai He, Brian J. Orr, Mitsuhiko Kono, and K. G. H. Baldwinhttp://www.opticsinfob...
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