Enhancing the functional properties of acetylated hemicellulose films for active food packaging using acetylated nanocellulose reinforcement and polycaprolactone coating

CITATION: Mugwagwa, L. R. & Chimphango, A. F. A. 2020. Enhancing the functional properties of acetylated hemicellulose films for active food packaging using acetylated nanocellulose reinforcement and polycaprolactone coating. Food Packaging and Shelf Life, 24. doi:10.1016/j.fpsl.2020.100481The original publication is available at https://www.sciencedirect.com/journal/food-packaging-and-shelf-lifeAcetylated hemicellulose (AH)-nanocellulose (ACNC) films coated with polycaprolactone (PCL) films, were evaluated as active packaging for aqueous, alcoholic, fatty and acidic food. The effects of nanocellulose loading (0–50 %), degree of acetylation (DS) (0–2.34) and polycaprolactone coating (0.3 g/mL) on hydrophobicity and solubility of AH films in food simulants, were investigated. In addition, AH-CNC/PCL films were doped with polyphenols and their antioxidant release (temperature 5 °C–40 °C, time - 48 h) into food simulants was evaluated experimentally and by modelling (Migratest software). Increasing ACNC DS and loading, combined with a PCL coating increased films’ hydrophobicity (24.59° to 82.48°) and reduced film solubility in all the simulants (∼82.8 %). The release of polyphenols by the films was highest and best predicted using Migratest software for the fatty food simulant. Therefore, these films can be used as active packaging for fatty foods. Furthermore, Migratest modelling can be used to predict film performance during film design.https://www.sciencedirect.com/science/article/pii/S221428941930496XPublishers versio