Magnetic Breakdown and Topology in the Kagome Superconductor CsV3Sb5 under High Magnetic Field

28 pages, 10 figures, 1 table, Supplementary Materials addedThe recently discovered layered Kagome metals of composition AV3Sb5 (A = K, Rb, Cs) exhibit a complex interplay among superconductivity, charge density wave order, topologically non-trivial electronic band structure and geometrical frustration. Here, we probe the electronic band structure underlying these exotic correlated electronic states in CsV3Sb5 with quantum oscillation measurements in pulsed fields up to 86 T. The high-field data reveal a sequence of magnetic breakdown orbits that allows the construction of a model for the folded Fermi surface of CsV3Sb5. The dominant features are large triangular Fermi surface sheets that cover almost half of the folded Brillouin zone that have not yet been detected in angle resolved photoemission spectroscopy (ARPES). These sheets display pronounced nesting at the charge density wave (CDW) vectors, which may stabilize the CDW state. The Berry phases of the electron orbits have been deduced from Landau level fan diagrams near the quantum limit without the need for extrapolations, thereby unambiguously establishing the non-trivial topological character of several electron bands in this Kagome lattice superconductor