Multiphoton k -resolved photoemission from gold surface states with 800-nm femtosecond laser pulses

  • Sirotti, Fausto
  • Beaulieu, Nathan
  • Bendounan, Azzedine
  • Silly, Mathieu G.
  • Chauvet, Christian
  • Malinowski, Grégory
  • Fratesi, Guido
  • Véniard, Valérie
  • Onida, Giovanni
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Publication date
January 2014
Publisher
American Physical Society (APS)

Abstract

International audienceWe measure direct multiphoton photoemission of the Au(111) surface state with 800-nm laser pulses. We observe the parabolic dispersion in the angular distribution of photoelectrons having absorbed between four and seven photons. The k dispersion we measure can be explained in terms of Shockley-state replicas, with a nascent hot electrons distribution at k above the Fermi level. Moderate laser power densities, of the order of 100 GW/cm 2 , resulted in large electron yields, indicating the importance of multiphoton excitations to define the electronic and magnetic properties of matter in the first hundred femtoseconds after laser excitation

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