International audienceIn this paper, second in this series, we discuss the nature of 66 faint carbon (C) stars which have been discovered by scrutinizing the plates of the First Byurakan Survey (FBS). These plates display lowresolution spectra of objects located at high Galactic latitudes and have a limiting magnitude of about V = 16. Our sample of 66 objects is part of a total of 120 stars found in the FBS and confirmed spectroscopically to be C stars. These 66 objects are those which show early-type spectra (not N-type). To better characterize these objects, medium-resolution CCD spectra were obtained and are exploited for them all, together with consideration of their 2MASS near-infrared (NIR) colors and their optical variability. First,...