International audienceThere is a deep connection between cosmology -- the science of the infinitely large --and particle physics -- the science of the infinitely small. This connection is particularly manifest in neutron particle physics. Basic properties of the neutron -- its Electric Dipole Moment and its lifetime -- are intertwined with baryogenesis and nucleosynthesis in the early Universe. I will cover this topic in the first part, that will also serve as an introduction (or rather a quick recap) of neutron physics and Big Bang cosmology. Then, the rest of the manuscript will be devoted to a new idea: using neutrons to probe models of Dark Energy. In the second part, I will present the chameleon theory: a light scalar field accounting ...