International audienceTo date, battery research largely follows an ``Edisonian'' approach based on experimental trial-and-error in contrast to a systematic strategy of design-of-experiments. Battery interfaces are arguably the most important yet the least understood components of energy storage devices. To transform the way we perform battery research, theory and computations can be used simultaneously to understand and guide the design of meaningful and targeted experiments. However, it is well known that modelling of battery interfaces is computationally prohibitive in terms of both resources and time due to the large size of systems to provide realistic and descriptive models. Recently, automated and intelligent in silico tools have been...