We revisit Vafa-Witten theory in the more general setting whereby the underlying moduli space is not that of instantons, but of the full Vafa-Witten equations. We physically derive (i) a novel Vafa-Witten four-manifold invariant associated with this moduli space, (ii) their relation to Gromov-Witten invariants, (iii) a novel Vafa-Witten Floer homology assigned to three-manifold boundaries, (iv) a novel Vafa-Witten Atiyah-Floer correspondence, (v) a proof and generalization of a conjecture by Abouzaid-Manolescu in [1] about the hypercohomology of a perverse sheaf of vanishing cycles, (vi) a Langlands duality of these invariants, Floer homologies and hypercohomology, and (vii) a quantum geometric Langlands correspondence with purely imaginary...