Tracking electron motion in molecules is the key to understanding and controlling chemical transformations. Contemporary techniques in attosecond science are able to generate and trace the consequences of this motion in real time, but not in real space. Scanning tunnelling microscopy, on the other hand, can locally probe the valence electron density in molecules, but cannot alone provide dynamical information at this ultrafast timescale. Here we show that, by combining scanning tunnelling microscopy and attosecond technologies, quantum electronic coherences induced in molecules by <6-fs-long carrier-envelope-phase-stable near-infrared laser pulses can be directly visualized at angstrom-scale spatial and subfemtosecond temporal resolutions. ...
This work introduces two experimental approaches to control quantum dynamics in molecules, employing...
The chemical properties of atoms, molecules and of more complex systems such as clusters, nanopartic...
International audienceThe many-body quantum nature of molecules determines their static and dynamic ...
Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural...
International audienceA strong laser field may tunnel ionize a molecule from several orbitals simult...
Watching a single molecule move on its intrinsic timescale has been one of the central goals of mode...
Time-resolved diffraction and microscopy with femtosecond electron pulses provide four-dimensional r...
We investigate theoretically the direct imaging of coherent electronic motion in atoms and molecules...
Author Institution: Department of Physics, The Ohio State University, Columbus, OH 43210; Department...
For the past several decades, we have been able to directly probe the motion of atoms that is associ...
We investigate theoretically the direct imaging of coherent electronic motion in atoms and molecules...
We demonstrate that an electron wave packet produced during intense field ionization can be used for...
Due to the important roles played by the electrons in various kinds of reactions, direct imaging ele...
This work introduces two experimental approaches to control quantum dynamics in molecules, employing...
The chemical properties of atoms, molecules and of more complex systems such as clusters, nanopartic...
International audienceThe many-body quantum nature of molecules determines their static and dynamic ...
Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural...
International audienceA strong laser field may tunnel ionize a molecule from several orbitals simult...
Watching a single molecule move on its intrinsic timescale has been one of the central goals of mode...
Time-resolved diffraction and microscopy with femtosecond electron pulses provide four-dimensional r...
We investigate theoretically the direct imaging of coherent electronic motion in atoms and molecules...
Author Institution: Department of Physics, The Ohio State University, Columbus, OH 43210; Department...
For the past several decades, we have been able to directly probe the motion of atoms that is associ...
We investigate theoretically the direct imaging of coherent electronic motion in atoms and molecules...
We demonstrate that an electron wave packet produced during intense field ionization can be used for...
Due to the important roles played by the electrons in various kinds of reactions, direct imaging ele...
This work introduces two experimental approaches to control quantum dynamics in molecules, employing...
The chemical properties of atoms, molecules and of more complex systems such as clusters, nanopartic...
International audienceThe many-body quantum nature of molecules determines their static and dynamic ...