Influence of Surface and Atmospheric Thermodynamic Properties on the Cloud Radiative Forcing and Radiative Energy Budget in the Arctic

The Arctic climate has changed significantly in the last decades, experiencing a dramatic loss of sea ice and stronger than global warming. The Arctic surface temperature and the growth or melt of sea ice is determined by the local surface energy budget. In this context, clouds are of essential importance as they strongly interact with the radiative fluxes and modulate the surface energy budget depending on their properties, the surface types, and atmospheric thermodynamics. For the quantification of changes in the radiative energy budget (REB) associated with the presence or absence of clouds, the concept of cloud radiative forcing (CRF) is commonly used. This concept is defined as the differences between the REB in cloudy and cloud-free conditions, two atmospheric states which can not be observed at the same location and time. Consequently, either radiative transfer simulations or observations in both states have to be related, both of which complicate the derivation of CRF. A review of available studies and their approaches to derive the CRF reveals conceptual differences as well as deficiencies in the handling of radiative processes related to the surface albedo. These findings call into question the current state of CRF assessment in the Arctic based on the few available studies, but also their comparability. By combining atmospheric radiative transfer simulations with a snow albedo model, two processes that control the surface albedo during the transition from cloud-free to cloudy conditions and their role in the derivation of CRF are discussed. The broadband surface albedo of snow surfaces typically increases in the presence of clouds due to a spectral weighting of downward irradiance toward shorter wavelengths. For more absorbing surface types such as white ice and melt ponds, which are common in summer, there is a strong shift between the albedo of direct and diffuse illuminated surface, which diminishes the surface albedo depending on the cloud optical thickness and solar zenith angle. In this thesis, a hypothesis on the impact of those surface-albedo--cloud interactions on the annual cycle of shortwave CRF is discussed, but an application to inner Arctic conditions remains an open issue. An improved method to derive the shortwave CRF is proposed and an application to two airborne campaigns in the marginal sea ice zone northwest of Svalbard (Norway) illustrates the role of surface-albedo--cloud interactions in the Arctic in spring and early summer. For the longwave CRF, conceptual differences and the general interpretation of the different CRF estimates are discussed and illustrated for a case study. Radiative transfer simulations of a rarely observed annual cycle of thermodynamic profiles in the inner Arctic are used to study both longwave CRF approaches and the impact of thermodynamic profiles on the longwave CRF. Making use of airborne low-level flights in the MIZ and other available datasets, common seasonal radiative states on sea ice and case studies of warm air intrusions and cold air outbreaks are illustrated. The CRF is analyzed as a function of the observed cloud/surface regime, which is extended by radiative transfer simulations characterizing the conditions in this region and seasons