To improve the high brittleness of recycled aggregate concrete containing iron ore tailings (TRAC), the feasibility of adding polypropylene fiber (PPF) to TRAC was studied by performing a compression stress–strain curve test, scanning electron microscope characterization, and a freeze–thaw cycle test. The results indicated that PPF had a beneficial impact on reducing the brittleness of TRAC. With the increase in PPF content, the peak strain increased, the elastic modulus decreased, and the peak stress and energy absorption capacity increased at first and then decreased. Furthermore, the microstructure investigation revealed that the interface friction between the PPF, aggregate, and cement matrix was the main source of energy dissipation. W...