This work was supported by the UK Space Agency (ST/P001297/1 and ST/P001394/1). AUPE3 data are available from http://exomars.wales.A key goal of the ExoMars rover Rosalind Franklin is to analyze accessible hydrated mineral deposits using panoramic multiscale and multispectral imagery. We conducted a multiscale spectroscopic study on hydrothermally-altered basalt-hosted soils in the geothermal area of Námafjall in northern Iceland. Basaltic lavas here that have experienced first-order geochemical alteration produce a variety of cm-to-meter scale poorly-crystalline alteration patterns. The resulting unconsolidated sediments provide a natural analogue material to investigate intimately mixed soils comprising multiple poorly-crystalline hydrate...