A DMI Guide to Magnets Micro-World

Abstract: Dzyaloshinskii–Moriya interaction, DMI in short, represents an antisymmetric type of magnetic interactions that favor orthogonal orientation of spins and competes with Heisenberg exchange. Being introduced to explain weak ferromagnetism in antiferromagnets without an inversion center between magnetic atoms such an anisotropic interaction can be used to analyze other non-trivial magnetic structures of technological importance including spin spirals and skyrmions. Despite the fact that the corresponding DMI contribution to the magnetic energy of the system has a very compact form of the vector product of spins, the determination of DMI from first-principles electronic structure is a very challenging methodological and technical problem whose solution opens a door into the fascinating microscopic world of complex magnetic materials. In this paper we review a few such methods developed by us for calculating DMI and their applications to study the properties of real materials. © 2021, Pleiades Publishing, Inc.The work of A.I.L. and M.I.K. is supported by European Research Council via Synergy Grant 854843-FASTCORR. Y.O.K. acknowledges the financial support from the Swedish Research Council (VR) under the project no. 2019-03569. The work of V.V.M. was supported by Act 211 Government of the Russian Federation, contract 02.A03.21.0006