Impact of dual-layer solid-electrolyte interphase inhomogeneities on early-stage defect formation in Si electrodes
- Chunguang Chen
- Tao Zhou
- Dmitri L. Danilov
- Lu Gao
- Svenja Benning
- Nino Schön
- Samuel Tardif
- Hugh Simons
- Florian Hausen
- Tobias U. Schülli
- R.-A. Eichel
- Peter H. L. Notten
Publication date
July 2020
DOI Publisher
Springer Science and Business Media LLC Journal
Nature CommunicationsAbstract
Severe structural deformation during (de)lithiation is the main factor limiting the stability of Si anodes in Li-ion batteries. Here, a multi-modal approach is used to visualize these deformations in their early-stage and link them to inhomogeneities in the dual-layer solid-electrolyte interphase
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