This dissertation comprises three essays in Econometrics and Political Economy offering both methodological and substantive contributions to the study of electoral coalitions (Chapter 2), the effectiveness of campaign expenditures (Chapter 3), and the general practice of experimentation (Chapter 4). Chapter 2 presents an empirical investigation of coalition formation in elections. Despite its prevalence in most democracies, there is little evidence documenting the impact of electoral coalition formation on election outcomes. To address this imbalance, I develop and estimate a structural model of electoral competition that enables me to conduct counterfactual analyses of election outcomes under alternative coalitional scenarios. The resul...