A narrowband, time-asymmetric probe pulse is introduced into the hybrid femtosecond/picosecond rotational coherent anti-Stokes Raman scattering (fs/ps RCARS) technique to provide accurate and precise single-shot, high-repetition-rate gas-phase thermometric measurements. This narrowband pulse-generated by inserting a Fabry-Pérot étalon into the probe-pulse beam path-enables frequency-domain detection of pure-rotational transitions. The unique time-asymmetric nature of this pulse, in turn, allows for detection of resonant Raman-active rotational transitions free of signal contamination by nonresonant four-wave-mixing processes while still allowing detection at short probe-pulse delays, where collisional dephasing processes are negligible. We ...
Coherent spectroscopy such as Coherent Anti-Stokes Raman Scattering (CARS) is commonly used for the ...
Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) is developed for me...
L'utilisation de techniques de spectroscopie cohérente comme la diffusion Raman anti-Stokes cohérent...
High-repetition-rate, single-laser-shot measurements are important for the investigation of unsteady...
Rotational-level-dependent dephasing rates and nonresonant background can lead to significant uncert...
A method for simultaneous ro-vibrational and pure-rotational hybrid femtosecond/picosecond coherent ...
Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) offers accurate the...
This paper was published in Optics Letters and is made available as an electronic reprint with the p...
The hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) technique prese...
We demonstrate hybrid femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman scattering for high-...
Gas-phase temperatures and concentrations are measured from the magnitude and decay of the initial R...
The direct measurement of self-broadened linewidths using the time decay of pure-rotational hybrid f...
A novel technique for studies of the dynamics of molecular coherences has been developed. The concep...
High-speed flows are important for defense, national security, and transportation applications and...
Hybrid fs/ps coherent anti-Stokes Raman CARS is a powerful laser diagnostic technique for thermometr...
Coherent spectroscopy such as Coherent Anti-Stokes Raman Scattering (CARS) is commonly used for the ...
Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) is developed for me...
L'utilisation de techniques de spectroscopie cohérente comme la diffusion Raman anti-Stokes cohérent...
High-repetition-rate, single-laser-shot measurements are important for the investigation of unsteady...
Rotational-level-dependent dephasing rates and nonresonant background can lead to significant uncert...
A method for simultaneous ro-vibrational and pure-rotational hybrid femtosecond/picosecond coherent ...
Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) offers accurate the...
This paper was published in Optics Letters and is made available as an electronic reprint with the p...
The hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) technique prese...
We demonstrate hybrid femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman scattering for high-...
Gas-phase temperatures and concentrations are measured from the magnitude and decay of the initial R...
The direct measurement of self-broadened linewidths using the time decay of pure-rotational hybrid f...
A novel technique for studies of the dynamics of molecular coherences has been developed. The concep...
High-speed flows are important for defense, national security, and transportation applications and...
Hybrid fs/ps coherent anti-Stokes Raman CARS is a powerful laser diagnostic technique for thermometr...
Coherent spectroscopy such as Coherent Anti-Stokes Raman Scattering (CARS) is commonly used for the ...
Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) is developed for me...
L'utilisation de techniques de spectroscopie cohérente comme la diffusion Raman anti-Stokes cohérent...