This article proposes a new road toll-design model for congested road networks with uncertain demand that can be used to create a sustainable urban transportation system. For policy assessment and strategic planning purposes, the proposed model extends traditional congestion pricing models to simultaneously consider congestion and environmental externalities due to vehicular use. Based on analyses of physical and environmental capacity constraints, the boundary conditions under which a road user on a link should pay either a congestion toll or an extra environmental tax are identified. The sustainable toll design model is formulated as a two-stage robust optimization problem. The first-stage problem before the realization of the future trav...