Nuclear motion driven by the Renner-Teller effect as observed in the resonant Auger decay to the X̃2Π electronic ground state of N2O+
- Miron, C.
- Simon, M.
- Morin, P.
- Nanbu, S.
- Kosugi, N.
- Sorensen, S. L.
- Naves De Brito, A.
- Piancastelli, M. N.
- Björneholm, O.
- Feifel, R.
- Bässler, M.
- Svensson, S.
DOIAbstract
The nuclear dynamics in the Nt 1s→π* in nitrous oxide was studied using the high resolution resonant Auger spectroscopy and ab initio quantum chemical calculations. For probing the nuclear motion of the system in the core-excited state, the frequency detuning technique was used. The results showed changes in vibrational structure for the Auger decay spectra and a strong influence of nuclear motion on the electronic decay
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