International audienceLand use change and the concomitant acceleration of soil erosion have led to an increase in sediment supply to rivers worldwide. This degradation results in significant on-site (e.g., decrease in soil fertility) and off-site impacts (e.g., reservoir siltation and degradation of water quality). To implement effective sediment mitigation measures, it is necessary to clearly understand catchment sediment sources and their spatial temporal dynamics. Fallout radionuclides characterized by different half-lives and origins (Be-7-53 d; Pb-210-22 y; Cs-137-30 y) provide important information required to quantify the dominant sources of sediment and also their temporal dynamics. However, the current methods have several limitati...