We investigate the perturbation and subsequent recovery of the correlated electronic ground state of the Mott insulator $\mathrm{1T-TaS_2}$ by means of femtosecond time-resolved photoemission spectroscopy in normal emission geometry. Upon an increase of near-infrared excitation strength, a considerable collapse of the occupied Hubbard band is observed, which reflects a quench of short-range correlations. It is furthermore found that these excitations are directly linked to the lifting of the periodic lattice distortion which provides the localization centers for the formation of the insulating Mott state. We discuss the observed dynamics in a localized real-space picture
The time-resolved determination of dynamics in complex materials is an important goal for understand...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
We investigate the perturbation and subsequent recovery of the correlated electronic ground state of...
Photoexcitation of the Mott insulator 1T-TaS2 by an intense laser pulse leads to an ultrafast transi...
Photoexcitation of the Mott insulator 1T-TaS2 by an intense laser pulse leads to an ultrafast transi...
Photoexcitation of the Mott insulator 1T-TaS2 by an intense laser pulse leads to an ultrafast transi...
The two-dimensional transition-metal dichalcogenide 1T−TaS2 is a complex material standing out for i...
Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic inter...
Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic intera...
Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic intera...
By using nearly-single-cycle optical pulses in the near infrared, we measure the time-dependent opti...
The time-resolved determination of dynamics in complex materials is an important goal for understand...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
The time-resolved determination of dynamics in complex materials is an important goal for understand...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
We investigate the perturbation and subsequent recovery of the correlated electronic ground state of...
Photoexcitation of the Mott insulator 1T-TaS2 by an intense laser pulse leads to an ultrafast transi...
Photoexcitation of the Mott insulator 1T-TaS2 by an intense laser pulse leads to an ultrafast transi...
Photoexcitation of the Mott insulator 1T-TaS2 by an intense laser pulse leads to an ultrafast transi...
The two-dimensional transition-metal dichalcogenide 1T−TaS2 is a complex material standing out for i...
Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic inter...
Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic intera...
Strongly correlated materials exhibit intriguing properties caused by intertwined microscopic intera...
By using nearly-single-cycle optical pulses in the near infrared, we measure the time-dependent opti...
The time-resolved determination of dynamics in complex materials is an important goal for understand...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
The time-resolved determination of dynamics in complex materials is an important goal for understand...
Competition between electron localization and delocalization in Mott insulators underpins the physic...
Competition between electron localization and delocalization in Mott insulators underpins the physic...