Glasses are inherently out-of-equilibrium systems evolving slowly toward their equilibrium state in a process called physical aging. During aging, dynamic observables depend on the history of the system, hampering comparative studies of dynamics in different glass formers. Here, we demonstrate how glass formers can be directly compared on the level of single-particle jumps, i.e. the structural relaxation events underlying the α-process. Describing the dynamics in terms of a continuous-time random walk, an analytic prediction for the jump rate is derived. The result is subsequently compared to molecular-dynamics simulations of amorphous silica and a polymer melt as two generic representatives of strong and fragile glass formers, and good agr...
Many fascinating questions still remain unsettled for condensed matter physicists who study the glas...
On approaching the glass transition, the microscopic kinetic unit spends increasing time rattling in...
50 pages, 24 figs. This is an updated version of a chapter initially written in 2009 for the Encyclo...
Glasses are inherently out-of-equilibrium systems evolving slowly toward their equilibrium state in ...
On cooling toward the glass transition temperature, glass-forming liquids display long periods of lo...
Non-equilibrium dynamics in the glassy state lead to interesting aging and memory effects. In this d...
Using molecular simulations, we identify microscopic relaxation events of individual particles in ag...
A popular picture of the intermittent dynamics of glassy materials depicts each particle as localize...
Particles in structural glasses rattle around temporary equilibrium positions, that seldom change th...
We investigate the aging dynamics of amorphous SiO2 via molecular dynamics simulations of a quench f...
The dynamical facilitation scenario, by which localized relaxation events promote nearby relaxation ...
We have studied, using dynamical Monte Carlo methods, a facilitated kinetic Ising model for structur...
The evaluation of the long term stability of a material requires the estimation of its long-time dyn...
If liquids, polymers, bio-materials, metals and molten salts can avoid crystallization during coolin...
68 pages; 21 figs; 481 references Journal: Rev. Mod. Phys. 83, 587 (2011)We provide a theoretical pe...
Many fascinating questions still remain unsettled for condensed matter physicists who study the glas...
On approaching the glass transition, the microscopic kinetic unit spends increasing time rattling in...
50 pages, 24 figs. This is an updated version of a chapter initially written in 2009 for the Encyclo...
Glasses are inherently out-of-equilibrium systems evolving slowly toward their equilibrium state in ...
On cooling toward the glass transition temperature, glass-forming liquids display long periods of lo...
Non-equilibrium dynamics in the glassy state lead to interesting aging and memory effects. In this d...
Using molecular simulations, we identify microscopic relaxation events of individual particles in ag...
A popular picture of the intermittent dynamics of glassy materials depicts each particle as localize...
Particles in structural glasses rattle around temporary equilibrium positions, that seldom change th...
We investigate the aging dynamics of amorphous SiO2 via molecular dynamics simulations of a quench f...
The dynamical facilitation scenario, by which localized relaxation events promote nearby relaxation ...
We have studied, using dynamical Monte Carlo methods, a facilitated kinetic Ising model for structur...
The evaluation of the long term stability of a material requires the estimation of its long-time dyn...
If liquids, polymers, bio-materials, metals and molten salts can avoid crystallization during coolin...
68 pages; 21 figs; 481 references Journal: Rev. Mod. Phys. 83, 587 (2011)We provide a theoretical pe...
Many fascinating questions still remain unsettled for condensed matter physicists who study the glas...
On approaching the glass transition, the microscopic kinetic unit spends increasing time rattling in...
50 pages, 24 figs. This is an updated version of a chapter initially written in 2009 for the Encyclo...