We investigate the dynamics of band occupation in gold after excitation with short laser pulses. Strong non‐equilibrium distributions can be created by intra‐ and inter‐band transitions driven by the absorption of photons with different wavelengths. First, we briefly discuss how photons can be used as a probe and how electrons with non‐Fermi distributions can be described. Then we focus on the relaxation stage where a temperature has been established but the occupation numbers in the different bands are not yet in equilibrium with this newly established elevated temperature. We describe the relaxation towards a system with a common chemical potential with rate equations that also include the energy transfer to the lattice or ions. Finally, ...
ultrafast absorption ; umklapp electron-electron collision ; collisional absorption ; laser-matter i...
Abstract: This paper describes our recent work using ultrafast laser spectroscopy to examine the fun...
ManuscriptWe propose a kinetic model of transient nonequilibrium phenomena in metals exposed to ultr...
Free electron lasers offer unique properties to study matter in states far from equilibrium as they ...
Intense ultrashort laser pulses can create highly excited matter with extraordinary properties. Expe...
Second-harmonic radiation is generated at a gold surface by use of a laser pulse that is varied in d...
In a thermally equilibrated system, electron behavior in a metal is described by the Fermi-Dirac equ...
Electron-phonon coupling is a fundamental process that governs the energy relaxation dynamics of sol...
International audienceWe investigate the nonlinear optical response of thin gold films with an unpre...
The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measu...
Thedirect assessment of the ultrafast temperature evolution of metallic nano-objects irradiated by a...
In this paper, we report on the Boltzmann kinetic equation approach adapted for simulations of warm ...
©1999 American Institute of Physics. The electronic version of this article is the complete one and ...
International audienceThe electronic behavior of various solid metals (Al, Ni, Cu, Au, Ti, and W) un...
Copyright © 2007 The American Physical SocietyUsing a supercontinuum pulse as a probe, we have measu...
ultrafast absorption ; umklapp electron-electron collision ; collisional absorption ; laser-matter i...
Abstract: This paper describes our recent work using ultrafast laser spectroscopy to examine the fun...
ManuscriptWe propose a kinetic model of transient nonequilibrium phenomena in metals exposed to ultr...
Free electron lasers offer unique properties to study matter in states far from equilibrium as they ...
Intense ultrashort laser pulses can create highly excited matter with extraordinary properties. Expe...
Second-harmonic radiation is generated at a gold surface by use of a laser pulse that is varied in d...
In a thermally equilibrated system, electron behavior in a metal is described by the Fermi-Dirac equ...
Electron-phonon coupling is a fundamental process that governs the energy relaxation dynamics of sol...
International audienceWe investigate the nonlinear optical response of thin gold films with an unpre...
The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measu...
Thedirect assessment of the ultrafast temperature evolution of metallic nano-objects irradiated by a...
In this paper, we report on the Boltzmann kinetic equation approach adapted for simulations of warm ...
©1999 American Institute of Physics. The electronic version of this article is the complete one and ...
International audienceThe electronic behavior of various solid metals (Al, Ni, Cu, Au, Ti, and W) un...
Copyright © 2007 The American Physical SocietyUsing a supercontinuum pulse as a probe, we have measu...
ultrafast absorption ; umklapp electron-electron collision ; collisional absorption ; laser-matter i...
Abstract: This paper describes our recent work using ultrafast laser spectroscopy to examine the fun...
ManuscriptWe propose a kinetic model of transient nonequilibrium phenomena in metals exposed to ultr...