Evaporative cooling of helium nanodroplets is studied with a statistical rate model that includes, for the first time, angular momentum conservation as a constraint on the accessible droplet states. It is found that while the final temperature of the droplets is almost identical to that previously predicted and later observed, the distribution of total droplet energy and angular momentum states is vastly more excited than a canonical distribution at the same temperature. It is found that the final angular momentum of the droplets is highly correlated with the initial direction, and that a significant fraction of the alignment of the total angular momentum should be transferred to the rotational angular momentum of an embedded molecule
International audienceThe clustering, collision, and relaxation dynamics of pristine and doped heliu...
Author Institution: Department, Princeton UniversitySuperfluid $^{4}He$ nanodroplets provide a novel...
$^{a}$C. Callegari, A. Conjusteau, I. Reinhard, K.K. Lehman, G. Scoles, and F. Dalfovo, Phys. Rev. L...
Author Institution: Department of Chemistry, Princeton UniversityIt is now well established experime...
Author Institution: Department of Chemistry, University of VirginiaThe rotational spectra of molecul...
Author Institution: Department of Chemistry, Princeton UniversityVortex lines, with quantized vortic...
We combine experimental and theoretical approaches to explore excited rotational states of molecules...
The feasibility of using rotating molecules as “nanoprobes” for testing the superfluidity of helium ...
While experiments and continuum models have provided a relatively good understanding of the evaporat...
Motivated by recent experiments, we study normal-phase rotating 3He droplets within density function...
We explore the collisional energy transfer dynamics of benzene molecules spontaneously evaporating f...
A new statistical model has been developed in the framework of Phase Space Theory to describe the ev...
In this introductory chapter, we begin by informing the reader about the fascinating history of supe...
Sublimation of a substance is the process of transitioning from solid phase to vapor phase. Despite ...
J.~Nagl, G.~Aubock, A.~W.~Hauser, O.~Allard, C.~Callegari, and W.~E.~Ernst, Phys.~Rev.~Lett. 100, ...
International audienceThe clustering, collision, and relaxation dynamics of pristine and doped heliu...
Author Institution: Department, Princeton UniversitySuperfluid $^{4}He$ nanodroplets provide a novel...
$^{a}$C. Callegari, A. Conjusteau, I. Reinhard, K.K. Lehman, G. Scoles, and F. Dalfovo, Phys. Rev. L...
Author Institution: Department of Chemistry, Princeton UniversityIt is now well established experime...
Author Institution: Department of Chemistry, University of VirginiaThe rotational spectra of molecul...
Author Institution: Department of Chemistry, Princeton UniversityVortex lines, with quantized vortic...
We combine experimental and theoretical approaches to explore excited rotational states of molecules...
The feasibility of using rotating molecules as “nanoprobes” for testing the superfluidity of helium ...
While experiments and continuum models have provided a relatively good understanding of the evaporat...
Motivated by recent experiments, we study normal-phase rotating 3He droplets within density function...
We explore the collisional energy transfer dynamics of benzene molecules spontaneously evaporating f...
A new statistical model has been developed in the framework of Phase Space Theory to describe the ev...
In this introductory chapter, we begin by informing the reader about the fascinating history of supe...
Sublimation of a substance is the process of transitioning from solid phase to vapor phase. Despite ...
J.~Nagl, G.~Aubock, A.~W.~Hauser, O.~Allard, C.~Callegari, and W.~E.~Ernst, Phys.~Rev.~Lett. 100, ...
International audienceThe clustering, collision, and relaxation dynamics of pristine and doped heliu...
Author Institution: Department, Princeton UniversitySuperfluid $^{4}He$ nanodroplets provide a novel...
$^{a}$C. Callegari, A. Conjusteau, I. Reinhard, K.K. Lehman, G. Scoles, and F. Dalfovo, Phys. Rev. L...