Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Luigi, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schroeter, C.
Moshammer, R.
Schlichting, I.
Joachim, U.
Rudenko, A.

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Open link

Publication date

January 2013

DOI

10.1103/PhysRevLett.110.053003

Publisher

American Physical Society (APS)

Language

English

Abstract

Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017 W/cm2) 5 fs x-ray pulses (ℏω=2 keV) are studied by coincident ion momentum spectroscopy. We contrast the measured charge state distribution with data on atomic Kr, determine kinetic energies of resulting ionic fragments, and compare them to the outcome of a Coulomb explosion model. We find signatures of ultrafast charge redistribution from the inner-shell ionized Se atom to its molecular partners, and observe significant displacement of the atomic constituents in the course of multiple ionization

Extracted data

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Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Luigi, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schroeter, C.
Moshammer, R.
Schlichting, I.
Joachim, U.
Rudenko, A.

Open PDF

Open link

Publication date

January 2013

DOI

10.1103/PhysRevLett.110.053003

Publisher

American Physical Society (APS)

Language

English

Abstract

Extracted data

Koji Motomura (1362552)
Edwin Kukk (1362576)
Hironobu Fukuzawa (1362594)
Shin-ichi Wada (1362540)
Kiyonobu Nagaya (1362588)
Satoshi Ohmura (1362591)
Subhendu Mondal (1362537)
Tetsuya Tachibana (1362573)
Yuta Ito (1362546)
Ryosuke Koga (1362570)
Tsukasa Sakai (1362564)
Kenji Matsunami (1362597)
Artem Rudenko (1362555)
Christophe Nicolas (1285563)
Xiao-Jing Liu (293521)
Catalin Miron (1285560)
Yizhu Zhang (1362549)
Yuhai Jiang (1362543)
Jianhui Chen (1362585)
Mailam Anand (1362600)
Dong Eon Kim (1362567)
Kensuke Tono (1362582)
Makina Yabashi (1362579)
Makoto Yao (1362561)
Kiyoshi Ueda (1362558)

December 2015

In recent years, free-electron lasers operating in the true X-ray regime have opened up access to th...

Coulomb explosion imaging of small polyatomic molecules with ultrashort x-ray pulses

Li, X.
Rudenko, A.
Schöffler, M.
Anders, N.
Baumann, T.
Eckart, S.
Erk, B.
Fanis, A.
Fehre, K.
Dörner, R.
Foucar, L.
Grundmann, S.
Grychtol, P.
Hartung, A.
Hofmann, M.
Ilchen, M.
Janke, C.
Kastirke, G.
Kircher, M.
Kubicek, K.
Kunitski, M.
Mazza, T.
Meister, S.
Melzer, N.
Montano, J.
Music, V.
Nalin, G.
Ovcharenko, Y.
Passow, C.
Pier, A.
Rennhack, N.
Rist, J.
Rivas, D.
Schlichting, I.
Schmidt, L.
Schmidt, P.
Siebert, J.
Strenger, N.
Trabert, D.
Trinter, F.
Vela-Perez, I.
Wagner, R.
Walter, P.
Weller, M.
Ziolkowski, P.
Czasch, A.
Rolles, D.
Meyer, M.
Jahnke, T.
Boll, R.

January 2022

Ultrashort x-ray pulses from free-electron lasers can efficiently charge up and trigger the full fra...

Overview of the spectrometer and the target injection setup in the CAMP chamber [43] used to perform coincident ion momentum spectroscopy on small organic molecules ionized with an x-ray FEL

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 1. Overview of the spectrometer and the target injection setup in the CAM...

Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules.

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Kupper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schroter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

February 2013

Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017 W/cm2) 5 fs x-ra...

Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Erk, Benjamin
Rolles, Daniel
Hundertmark, A.
Marchenko, T.
Simon, Marc
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Foucar, L.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schröter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, Artem
Rudek, Benedikt
Epp, Sascha
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.

January 2013

Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017 W/cm2) 5 fs x-ra...

Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schroeter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

February 2013

Ionization and fragmentation of methylselenol (CH(3)SeH) molecules by intense (>10(17) W/cm(2)) 5 fs...

Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schröter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

August 2013

The ionization and fragmentation of two selenium containing hydrocarbon molecules, methylselenol (CH...

Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging.

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schröter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

January 2013

The ionization and fragmentation of two selenium containing hydrocarbon molecules, methylselenol (CH...

The kinetic energy distributions of carbon ions for 'anomalous' fragmentation channels where carbon is charged higher than selenium

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 5. The kinetic energy distributions of carbon ions for 'anomalous' fragme...

The kinetic energy distributions of carbon ions for different fragmentation channels of methylselenol (a), (b) and ethylselenol (c), (d)

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 4. The kinetic energy distributions of carbon ions for different fragment...

(a) Ion time-of-flight spectra resulting from the ionization and fragmentation of methylselenol (CH3SeH) and ethylselenol (C2H5SeH) molecules by 5 fs-XFEL pulses with a nominal pulse energy of 0.4 mJ and a photon energy of 2.0 keV (methylselenol, red dashed line) and 1.7 keV (ethylselenol, blue solid line)

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 2. (a) Ion time-of-flight spectra resulting from the ionization and fragm...

Femtosecond Charge and Molecular Dynamics of I-containing organic molecules Induced by Intense X-Ray Free-Electron Laser Pulses

Nagaya, K
Motomura, K
Kukk, E
Takahashi, Y
Yamazaki, K
Ohmura, S
Fukuzawa, H
Wada, S
Mondal, S
Tachibana, T
Ito, Y
Koga, R
Sakai, T
Matsunami, K
Nakamura, K
Kanno, M
Rudenko, A
Nicolas, C
Liu, XJ
Miron, C
Zhang, Y
Jiang, Y
Chen, J
Anand, M
Kim, DE
Tono, K
Yabashi, M
Yao, M
Konoe, H
Ueda, K

February 2019

We studied the electronic and nuclear dynamics of I-containing organic molecules induced by intense ...

Charge and Nuclear Dynamics Induced by Deep Inner-Shell Multiphoton Ionization of CH3I Molecules by Intense X‑ray Free-Electron Laser Pulses

Koji Motomura (1362552)
Edwin Kukk (1362576)
Hironobu Fukuzawa (1362594)
Shin-ichi Wada (1362540)
Kiyonobu Nagaya (1362588)
Satoshi Ohmura (1362591)
Subhendu Mondal (1362537)
Tetsuya Tachibana (1362573)
Yuta Ito (1362546)
Ryosuke Koga (1362570)
Tsukasa Sakai (1362564)
Kenji Matsunami (1362597)
Artem Rudenko (1362555)
Christophe Nicolas (1285563)
Xiao-Jing Liu (293521)
Catalin Miron (1285560)
Yizhu Zhang (1362549)
Yuhai Jiang (1362543)
Jianhui Chen (1362585)
Mailam Anand (1362600)
Dong Eon Kim (1362567)
Kensuke Tono (1362582)
Makina Yabashi (1362579)
Makoto Yao (1362561)
Kiyoshi Ueda (1362558)

December 2015

In recent years, free-electron lasers operating in the true X-ray regime have opened up access to th...

Coulomb explosion imaging of small polyatomic molecules with ultrashort x-ray pulses

Li, X.
Rudenko, A.
Schöffler, M.
Anders, N.
Baumann, T.
Eckart, S.
Erk, B.
Fanis, A.
Fehre, K.
Dörner, R.
Foucar, L.
Grundmann, S.
Grychtol, P.
Hartung, A.
Hofmann, M.
Ilchen, M.
Janke, C.
Kastirke, G.
Kircher, M.
Kubicek, K.
Kunitski, M.
Mazza, T.
Meister, S.
Melzer, N.
Montano, J.
Music, V.
Nalin, G.
Ovcharenko, Y.
Passow, C.
Pier, A.
Rennhack, N.
Rist, J.
Rivas, D.
Schlichting, I.
Schmidt, L.
Schmidt, P.
Siebert, J.
Strenger, N.
Trabert, D.
Trinter, F.
Vela-Perez, I.
Wagner, R.
Walter, P.
Weller, M.
Ziolkowski, P.
Czasch, A.
Rolles, D.
Meyer, M.
Jahnke, T.
Boll, R.

January 2022

Ultrashort x-ray pulses from free-electron lasers can efficiently charge up and trigger the full fra...

Overview of the spectrometer and the target injection setup in the CAMP chamber [43] used to perform coincident ion momentum spectroscopy on small organic molecules ionized with an x-ray FEL

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 1. Overview of the spectrometer and the target injection setup in the CAM...

Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules.

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Kupper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schroter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

February 2013

Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017 W/cm2) 5 fs x-ra...

Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Erk, Benjamin
Rolles, Daniel
Hundertmark, A.
Marchenko, T.
Simon, Marc
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Foucar, L.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schröter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, Artem
Rudek, Benedikt
Epp, Sascha
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.

January 2013

Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017 W/cm2) 5 fs x-ra...

Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schroeter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

February 2013

Ionization and fragmentation of methylselenol (CH(3)SeH) molecules by intense (>10(17) W/cm(2)) 5 fs...

Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schröter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

August 2013

The ionization and fragmentation of two selenium containing hydrocarbon molecules, methylselenol (CH...

Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging.

Erk, B.
Rolles, D.
Foucar, L.
Rudek, B.
Epp, S.
Cryle, M.
Bostedt, C.
Schorb, S.
Bozek, J.
Rouzee, A.
Hundertmark, A.
Marchenko, T.
Simon, M.
Filsinger, F.
Christensen, L.
De, S.
Trippel, S.
Küpper, J.
Stapelfeldt, H.
Wada, S.
Ueda, K.
Swiggers, M.
Messerschmidt, M.
Schröter, C.
Moshammer, R.
Schlichting, I.
Ullrich, J.
Rudenko, A.

January 2013

The ionization and fragmentation of two selenium containing hydrocarbon molecules, methylselenol (CH...

The kinetic energy distributions of carbon ions for 'anomalous' fragmentation channels where carbon is charged higher than selenium

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 5. The kinetic energy distributions of carbon ions for 'anomalous' fragme...

The kinetic energy distributions of carbon ions for different fragmentation channels of methylselenol (a), (b) and ethylselenol (c), (d)

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 4. The kinetic energy distributions of carbon ions for different fragment...

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 2. (a) Ion time-of-flight spectra resulting from the ionization and fragm...

Femtosecond Charge and Molecular Dynamics of I-containing organic molecules Induced by Intense X-Ray Free-Electron Laser Pulses

Nagaya, K
Motomura, K
Kukk, E
Takahashi, Y
Yamazaki, K
Ohmura, S
Fukuzawa, H
Wada, S
Mondal, S
Tachibana, T
Ito, Y
Koga, R
Sakai, T
Matsunami, K
Nakamura, K
Kanno, M
Rudenko, A
Nicolas, C
Liu, XJ
Miron, C
Zhang, Y
Jiang, Y
Chen, J
Anand, M
Kim, DE
Tono, K
Yabashi, M
Yao, M
Konoe, H
Ueda, K

February 2019

We studied the electronic and nuclear dynamics of I-containing organic molecules induced by intense ...

Charge and Nuclear Dynamics Induced by Deep Inner-Shell Multiphoton Ionization of CH3I Molecules by Intense X‑ray Free-Electron Laser Pulses

Koji Motomura (1362552)
Edwin Kukk (1362576)
Hironobu Fukuzawa (1362594)
Shin-ichi Wada (1362540)
Kiyonobu Nagaya (1362588)
Satoshi Ohmura (1362591)
Subhendu Mondal (1362537)
Tetsuya Tachibana (1362573)
Yuta Ito (1362546)
Ryosuke Koga (1362570)
Tsukasa Sakai (1362564)
Kenji Matsunami (1362597)
Artem Rudenko (1362555)
Christophe Nicolas (1285563)
Xiao-Jing Liu (293521)
Catalin Miron (1285560)
Yizhu Zhang (1362549)
Yuhai Jiang (1362543)
Jianhui Chen (1362585)
Mailam Anand (1362600)
Dong Eon Kim (1362567)
Kensuke Tono (1362582)
Makina Yabashi (1362579)
Makoto Yao (1362561)
Kiyoshi Ueda (1362558)

December 2015

In recent years, free-electron lasers operating in the true X-ray regime have opened up access to th...

Coulomb explosion imaging of small polyatomic molecules with ultrashort x-ray pulses

Li, X.
Rudenko, A.
Schöffler, M.
Anders, N.
Baumann, T.
Eckart, S.
Erk, B.
Fanis, A.
Fehre, K.
Dörner, R.
Foucar, L.
Grundmann, S.
Grychtol, P.
Hartung, A.
Hofmann, M.
Ilchen, M.
Janke, C.
Kastirke, G.
Kircher, M.
Kubicek, K.
Kunitski, M.
Mazza, T.
Meister, S.
Melzer, N.
Montano, J.
Music, V.
Nalin, G.
Ovcharenko, Y.
Passow, C.
Pier, A.
Rennhack, N.
Rist, J.
Rivas, D.
Schlichting, I.
Schmidt, L.
Schmidt, P.
Siebert, J.
Strenger, N.
Trabert, D.
Trinter, F.
Vela-Perez, I.
Wagner, R.
Walter, P.
Weller, M.
Ziolkowski, P.
Czasch, A.
Rolles, D.
Meyer, M.
Jahnke, T.
Boll, R.

January 2022

Ultrashort x-ray pulses from free-electron lasers can efficiently charge up and trigger the full fra...

Overview of the spectrometer and the target injection setup in the CAMP chamber [43] used to perform coincident ion momentum spectroscopy on small organic molecules ionized with an x-ray FEL

B Erk (557608)
J Bozek (557615)
S Schorb (557614)
C Bostedt (557613)
M Cryle (557612)
S W Epp (557611)
B Rudek (557610)
L Foucar (557587)
D Rolles (557609)
A Rouzee (557616)

August 2013

Figure 1. Overview of the spectrometer and the target injection setup in the CAM...

Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Abstract

Extracted data

Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Abstract

Extracted data

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