Cooling of the Earth's mantle since the Meso-Archean is predicted by thermal and petrological models to have induced a secular change in the composition of primary mantle-derived magmas – and thus bulk oceanic crust; in particular, suggesting a decrease in maficity over time. This hypothesis underpins several recent studies that have addressed key geological questions concerning evolving plate tectonic styles, the rates and timing of continental crust formation, comparative planetology, and the emergence of complex life on Earth. Major, minor, and trace element geochemical analyses of (meta)mafic rocks preserved in the geological record allows exploration of this theory, although no consensus currently exists about the magnitude of this cha...