Design of efficient single-stage chirped pulse difference frequency generation at 7μm, driven by a dual wavelength Ti:sapphire laser

We present simulations for a design of a high-energy single-stage mid-IR difference frequency generation adapted to a two-color Ti:sapphire amplifier system. The optimized mixing process is based on chirped pulse difference frequency generation (CP-DFG), allowing for a higher conversion efficiency and reduced two-photon absorption losses. The numerical start-to-end simulations include stretching, chirped pulse difference frequency generation and pulse compression. Realistic design parameters for commercially available nonlinear crystals (GaSe, AgGaS2, LiInSe2, LiGaSe2) are considered. Compared with conventional unchirped DFG directly pumped by Ti:sapphire technology, we predict a threefold increase in the quantum efficiency. Our CP-DFG scheme provides up to 340μJ pulse energy directly at 7.2μm when pumped with 8mJ and supports a bandwidth of up to 350nm. The resulting 240fs mid-IR pulses are inherently phase stable