Meteorite cloudy zone formation as a quantitative indicator of paleomagnetic field intensities and cooling rates on planetesimals

Metallic microstructures in slowly-cooled iron-rich meteorites reflect the thermal and magnetic histories of their parent planetesimals. Of particular interest is the cloudy zone, a nanoscale intergrowth of Ni-rich islands within a Ni-poor matrix that forms below ∼350 °C by spinodal decomposition. The sizes of the islands have long been recognized as reflecting the low-temperature cooling rates of meteorite parent bodies. However, a model capable of providing quantitative cooling rate estimates from island sizes has been lacking. Moreover, these islands are also capable of preserving a record of the ambient magnetic field as they grew, but some of the key physical parameters required for recovering reliable paleointensity estimates from magnetic measurements of these islands have been poorly constrained. To address both of these issues, we present a numerical model of the structural and compositional evolution of the cloudy zone as a function of cooling rate and local composition. Our model produces island sizes that are consistent with present-day measured sizes. This model enables a substantial improvement in the calibration of paleointensity estimates and associated uncertainties. In particular, we can now accurately quantify the statistical uncertainty associated with the finite number of islands acquiring the magnetization and the uncertainty on their size at the time of the record. We use this new understanding to revisit paleointensities from previous pioneering paleomagnetic studies of cloudy zones. We show that these could have been overestimated by up to one order of magnitude but nevertheless still require substantial magnetic fields to have been present on their parent bodies. Our model also allows us to estimate absolute cooling rates for meteorites that cooled slower than