Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Nuclear Science and Engineering, February 2013."December 2012." Cataloged from PDF version of thesis.Includes bibliographical references (p. 145-160).Processing information quantum mechanically allows the relatively efficient solution of many important problems thought to be intractable on a classical computer. A primary challenge in experimentally implementing a quantum information processor is the control and suppression of environmental noise that decoheres the quantum system and causes it to behave classically. Environmental errors may be dynamically suppressed by applying coherent control pulses to the qubits that decouple the environment. However, the pulses themselves a...