Starting from an antiferromagnetic Heisenberg Hamiltonian for the 15 spin-1/2 ions in $V_{15}$, we construct an effective spin Hamiltonian involving eight low-lying states (spin-1/2 and spin-3/2) coupled to a phonon bath. We numerically solve the time-dependent Schrodinger equation of this system, and obtain the magnetization as a function of temperature in a time-dependent magnetic field. The magnetization exhibits unusual patterns of hysteresis and plateaus as the field sweep rate and temperature are varied. The observed plateaus are not due to quantum tunnelling but are a result of thermal averaging. Our results are in good agreement with recent experimental observations
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
Starting from an antiferromagnetic Heisenberg Hamiltonian for the 15 spin-½ ions in V15, we con...
Quantum tunneling of the magnetization (QTM) of the spin-1/2 Vanadium-15 (V15) single molecular magn...
We calculate the response of a molecular magnet subject to a time-varying magnetic field and coupled...
Beginning with a Heisenberg spin Hamiltonian for the manganese ions in the Mn12Ac molecule, we find ...
Beginning with a Heisenberg: spin Hamiltonian for the manganese ions in the Mn12Ac molecule, we find...
Beginning with a Heisenberg: spin Hamiltonian for the manganese ions in the Mn12Ac molecule, we find...
Chiorescu I, Wernsdorfer W, Müller A, Miyashita S, Barbara B. Adiabatic Landau-Zener-Stuckelberg tra...
Single-molecule magnets of the type V-15(K-6[V15As6O42(H2O)].8H(2)O) have attracted a great deal of ...
Contains fulltext : 60385.pdf (publisher's version ) (Open Access)Single-molecule ...
Chiorescu I, Wernsdorfer W, Müller A, Bögge H, Barbara B. Butterfly hysteresis loop and dissipative ...
Barbara B, Chiorescu I, Wernsdorfer W, Bögge H, Müller A. The V-15 molecule, a multi-spin two-level ...
We have observed hysteresis loops and abrupt magnetization steps in the magnetic molecule {V6}, wher...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
Starting from an antiferromagnetic Heisenberg Hamiltonian for the 15 spin-½ ions in V15, we con...
Quantum tunneling of the magnetization (QTM) of the spin-1/2 Vanadium-15 (V15) single molecular magn...
We calculate the response of a molecular magnet subject to a time-varying magnetic field and coupled...
Beginning with a Heisenberg spin Hamiltonian for the manganese ions in the Mn12Ac molecule, we find ...
Beginning with a Heisenberg: spin Hamiltonian for the manganese ions in the Mn12Ac molecule, we find...
Beginning with a Heisenberg: spin Hamiltonian for the manganese ions in the Mn12Ac molecule, we find...
Chiorescu I, Wernsdorfer W, Müller A, Miyashita S, Barbara B. Adiabatic Landau-Zener-Stuckelberg tra...
Single-molecule magnets of the type V-15(K-6[V15As6O42(H2O)].8H(2)O) have attracted a great deal of ...
Contains fulltext : 60385.pdf (publisher's version ) (Open Access)Single-molecule ...
Chiorescu I, Wernsdorfer W, Müller A, Bögge H, Barbara B. Butterfly hysteresis loop and dissipative ...
Barbara B, Chiorescu I, Wernsdorfer W, Bögge H, Müller A. The V-15 molecule, a multi-spin two-level ...
We have observed hysteresis loops and abrupt magnetization steps in the magnetic molecule {V6}, wher...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, u...