A random sample of 98 Gregorian chants was used to assemble “mode profiles”—pitch-class distributions for each of eight medieval modes in the manner of Krumhansl’s and Kessler’s (1982) key profiles. These profiles are shown to be useful in predicting the conventional modal designation for individual chants. An analysis of the eight mode profiles suggests that modes 3, 5 and 8 (Phrygian, Lydian and Hy-pomixolydian) are highly similar and can be distinguished from a more heterogeneous group consisting of the remaining modes. A cluster analysis of profiles for individual chants gives further evidence that these three modes form a supramodal category. The results are shown to be consistent with a theory of mode offered by the 11th-century...