Heat Capacity Reveals the Physics of a Frustrated Spin Tube

Ivanov N, Schnack J, Schnalle R, et al. Heat Capacity Reveals the Physics of a Frustrated Spin Tube. Physical Review Letters. 2010;105(3): 37206.We report on theoretical and experimental results concerning the low-temperature specific heat of the frustrated spin-tube material [(CuCl(2)tachH)(3)Cl]Cl-2 (tach denotes 1,3,5-triaminocyclohexane). This substance turns out to be an unusually perfect spin-tube system which allows to study the physics of quasione- dimensional antiferromagnetic structures in rather general terms. An analysis of the specific-heat data demonstrates that at low enough temperatures the system exhibits a Tomonaga-Luttinger liquid behavior corresponding to an effective spin-3/2 antiferromagnetic Heisenberg chain with short-range exchange interactions. On the other hand, around 2 K the composite spin structure of the chain is revealed through a Schottky-type peak in the specific heat. We argue that the dominating contribution to the peak originates from gapped magnon-type excitations related to the internal degrees of freedom of the rung spins