The Evolution of Springtime Water Vapor Over Beijing Observed by a High Dynamic Raman Lidar System: Case Studies

Raman lidar is an effective technique to retrieve the vertical distribution of atmospheric water vapor. For the first time, we present water vapor profiles retrieved by a high dynamic Raman lidar system over the Beijing area for representative cases in spring 2014, within the framework of the Aerosol Multi-wavelength Polarization Lidar Experiment project. In springtime, water vapor content over Beijing is generally low but with a strong daily variability. Its evolution is strongly coupled with winds and aerosols, with clouds also exerting a distinct impact. Northwesterly winds is found to be the most important factor impacting the temporal variability of water vapor mixing ratio (WVMR), and WVMR is found to be negatively correlated with wind speed. Moreover, we find that clouds tend to cause significant increases in the standard deviation of WMVR measurement, and relative humidity sharply increase below the cloud base. During a typical pollution episode, water vapor strongly covaries with aerosols due to hygroscopic growth effect and transport mechanism. Both water vapor and aerosols exhibit the highest variability within the planetary boundary layer (PBL), where the development and dissipation of haze mainly occur. Within the PBL, water vapor and aerosol concentration demonstrate different evolution features at different altitudes during the haze process, with a delayed increase and early decrease for higher altitudes. Back trajectory analysis using the hybrid single-particle Lagrangian trajectory model indicates that this phenomenon is most likely associated with different sources of the air mass at different altitudes.National Natural Science Foundation of China [41375008, 41175020]; "Strategic Priority Research Program" of the Chinese Academy of Sciences [XDA05040203]; President's Undergraduate Research Fellowship of Peking University; National High Technology Research and Development Program of China through the 863 Major Project [SQ2010AA1221583001]SCI(E)ARTICLE51715-17261