Inhalation exposure and risk of polycyclic aromatic hydrocarbons (PAHs) among the rural population adopting wood gasifier stoves compared to different fuel-stove users

Polycyclic aromatica hydrocarbons (PAHs) are a group of compounds with carcinogenic potentials and residential solid fuel combustion is one major source of PAHs in most developing countries. Replacement of traditional stoves with improved ones is believed to be a practical approach to reduce pollutant emissions, however, field assessments on the performance and consequent impacts on air quality and human health after adopting improved stoves are rare. The study is the first time to quantify inhalation exposure to PAHs among the residents who adopted wood gasifier stoves. The results were compared to those still burning coals in the region and compared to exposure levels for different fuel/stove users in literature. The results showed that the PAHs exposure levels for the wood gasifier stove users were significantly lower than the values for those using traditional wood stoves reported in literature, and the daily exposure concentrations of BaPeq (Benzo[a]pyrene equivalent concentration) can be reduced by 48% -91% if traditional wood stoves were replaced by wood gasifier stoves. The corresponding Incremental Lifetime Cancer Risk (ILCR) decreased approximately four times from 1.94 x 10(-4) to 5.17 x 10(-5). The average concentration of the total 26 PAHs for the wood users was 1091 +/- 722 ng/m(3), which was comparable to 1060 +/- 927 ng/m(3) for those using anthracite coals, but the composition profiles were considerably different. The average BaPeq were 116 and 25.8 ng/m(3) for the wood and coal users, respectively, and the corresponding ILCR of the anthracite coal users was 1.69 x 10(-5), which was nearly one third of those using the wood gasifier stoves. The wood users exposed to not only high levels of high molecular weight PAHs, but relatively high fractions of particulate phase PAHs in small particles compared to the coal users, resulting in high exposure risks. (C) 2016 Elsevier Ltd. All rights reserved.National Natural Science Foundation of China [41390240, 41130754, 41301554, 41571130010]; Ministry of Science and Technology [2015DFG92090]; Global Alliance for Clean StovesSCI(E)EISSCIARTICLEgqliu@mail.buct.edu.cn; taos@pku.edu.cn485-49114