Social computing systems, fueled by the ability of the Internet to engage millions of individuals, have redefined computation to include not only the application of algorithms but also the participation of people. Yet, the true impact of social computing in the future depends on a systematic understanding of how to design interventions that produce desirable system-wide behavior. Behavioral experiments, with their fundamental ability to study causality, are an important methodology in reaching this goal. This dissertation presents several examples of how novel experimental approaches to studying social computing systems can not only improve the design of such systems, but improve our understanding of human behavior. We investigate the diff...