This thesis describes structures of the quantum BRST constraint method in a mathematically rigorous manner by formulating it in a C*-algebraic context, leading to comparison of the quantum BRST and the Dirac constraint method in a rigorous manner.Rigorous models are constructed for the heuristic examples of BRST for quantum electromagnetism (BRST-QEM) and Hamiltonian BRST with a finite number of constraints. This facilitates comparison between the results produced by the BRST method, and the results of the T-procedure of Grundling and Hurst for the quantum Dirac constraint method.The different constraint methods are shown not to be equivalent for the examples of Hamiltonian BRST with a finite number of constraints that close, and a BRST-QEM...